Unraveling pairon excitations and the antiferromagnetic contributions in the cuprate specific heat
Abstract
Thermal measurements, such as the entropy and the specific heat, reveal key elementary excitations for understanding the cuprates. In this paper, we study the specific heat measurements on three different compounds La2-xSrxCuO4, Bi2Sr2CaCu2O 8+δ and YBa2Cu3O 7-δ and show that the data are compatible with 'pairons' and their excitations. However, the precise fits require the contribution of the antiferromagnetic entropy deduced from the magnetic susceptibility χ(T ).
Two temperature scales are involved in the excitations above the critical temperature Tc: the pseudogap T * , related to pairon excitations, and the magnetic correlation temperature, Tmax, having very different dependencies on the carrier density (p). In agreement with our previous analysis of χ(T ), the Tmax(p) line is not the signature of a gap in the electronic density of states, but is rather the temperature scale of strong local antiferromagnetic correlations which dominate for low carrier concentration. These progressively evolve into paramagnetic fluctuations in the overdoped limit.
Our results are in striking contradiction with the model of J. L. Tallon and J. G. Storey [Phys. Rev. B 107, 054507 (2023)], who reaffirm the idea of a T -independent gap Eg, whose temperature scale Tg = Eg/kB decreases linearly with p and vanishes at a critical value pc ∼ 0.19.
Finally, we discuss the unconventional fluctuation regime above Tc, which is associated with a mini-gap δ ∼ 2 meV in the pairon excitation spectrum. This energy scale is fundamental to the condensation mechanism.
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