Probing the Energy Conversion Pathways between Light, Carriers, and Lattice in Real Time with Attosecond Core-Level Spectroscopy - CNRS - Centre national de la recherche scientifique Accéder directement au contenu
Article Dans Une Revue Physical Review X Année : 2021

Probing the Energy Conversion Pathways between Light, Carriers, and Lattice in Real Time with Attosecond Core-Level Spectroscopy

B Bauerhenne
S Krylow
T Vasileiadis
Yves Joly
R Ernstorfer

Résumé

Detection of the energy conversion pathways, between photons, charge carriers, and the lattice is of fundamental importance to understand fundamental physics and to advance materials and devices. Yet, such insight remains incomplete due to experimental challenges in disentangling the various signatures on overlapping time scales. Here, we show that attosecond core-level X-ray spectroscopy can identify these interactions with attosecond precision and across a picosecond range. We demonstrate this methodology on graphite since its investigation is complicated by a variety of mechanisms occurring across a wide range of temporal scales. Our methodology reveals, through the simultaneous real-time detection of electrons and holes, the different dephasing mechanisms for each carrier type dependent on excitation with few-cycle-duration light fields. These results demonstrate the general ability of our methodology to detect and distinguish the various dynamic contributions to the flow of energy inside materials on their native time scales
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Dates et versions

hal-03505618 , version 1 (28-10-2021)
hal-03505618 , version 2 (04-11-2021)
hal-03505618 , version 3 (31-12-2021)

Identifiants

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T P H Sidiropoulos, N Di Palo, D E Rivas, S Severino, M Reduzzi, et al.. Probing the Energy Conversion Pathways between Light, Carriers, and Lattice in Real Time with Attosecond Core-Level Spectroscopy. Physical Review X, 2021, 11 (4), pp.041060. ⟨10.1103/physrevx.11.041060⟩. ⟨hal-03505618v3⟩

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