Improved constraints on hematite refractive index for estimating climatic effects of dust aerosols - CNRS - Centre national de la recherche scientifique
Article Dans Une Revue Communications Earth & Environment Année : 2024

Improved constraints on hematite refractive index for estimating climatic effects of dust aerosols

Longlei Li
Natalie Mahowald
María Gonçalves Ageitos
  • Fonction : Auteur
Vincenzo Obiso
  • Fonction : Auteur
Ron Miller
  • Fonction : Auteur
Carlos Pérez García-Pando
Philip Brodrick
  • Fonction : Auteur
Roger Clark
  • Fonction : Auteur
Robert Green
  • Fonction : Auteur
Raymond Kokaly
  • Fonction : Auteur
Gregg Swayze
  • Fonction : Auteur
David Thompson
  • Fonction : Auteur

Résumé

Abstract Uncertainty in desert dust composition poses a big challenge to understanding Earth’s climate across different epochs. Of particular concern is hematite, an iron-oxide mineral dominating the solar absorption by dust particles, for which current estimates of absorption capacity vary by over two orders of magnitude. Here, we show that laboratory measurements of dust composition, absorption, and scattering provide valuable constraints on the absorption potential of hematite, substantially narrowing its range of plausible values. The success of this constraint is supported by results from an atmospheric transport model compared with station-based measurements. Additionally, we identify substantial bias in simulating hematite abundance in dust aerosols with current soil mineralogy descriptions, underscoring the necessity for improved data sources. Encouragingly, the next-generation imaging spectroscopy remote sensing data hold promise for capturing the spatial variability of hematite. These insights have implications for enhancing dust modeling, thus contributing to efforts in climate change mitigation and adaptation.
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hal-04756971 , version 1 (29-10-2024)

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Longlei Li, Natalie Mahowald, María Gonçalves Ageitos, Vincenzo Obiso, Ron Miller, et al.. Improved constraints on hematite refractive index for estimating climatic effects of dust aerosols. Communications Earth & Environment, 2024, 5 (1), pp.295. ⟨10.1038/s43247-024-01441-4⟩. ⟨hal-04756971⟩
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